Cascade х(3)-nonlinear processes in new SRS active Ca2MgSi2O7 crystal

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Abstract

The observation of stimulated Raman scattering (SRS) in magnesium silicate Ca2MgSi2O7, entering the family of D32d-tetragonal acentric crystals with the structure of melilite, is reported. The registered components of the Stokes and anti-Stokes Χ(3)-nonlinear crystal lasing are identified with two active SRS‑modes ωSRS1 ≈ 908 cm1 and ωSRS2 ≈ 668 cm1, which also manifest in the generation of combined phonon modes ωSRS3C ≈ 170 cm1 and ωSRS4C ≈ 1270 cm1.

About the authors

A. A. Kaminskii

Shubnikov Crystallography Institute of the Russian Academy of Sciences

Author for correspondence.
Email: kaminalex@mail.ru

Corresponding Member of the Russian Academy of Sciences

Russian Federation, 59, Leninsky prospect, Moscow, 117333

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